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    Dimensional evolution of anisotropic magnetoresistance in MnBi2Te4

    K. Rao1, X. Zhang2,*, W. S. Hou1, M. Q. Dong1,3, Z. F. Dai1, Z. X. Song1, and Zhi-Xin Guo1,†

    • 1State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering, Xi'an Jiaotong University, Xi'an, Shaanxi 710049, China
    • 2Shaanxi Key Laboratory of Surface Engineering and Remanufacturing College of Mechanical and Materials Engineering, Xi'an University, Xi'an 710065, China
    • 3Key Laboratory of Computational Physical Sciences (Ministry of Education), Institute of Computational Physical Sciences, State Key Laboratory of Surface Physics, and Department of Physics, Fudan University, Shanghai 200433, China

    • *Contact author: zhangxian1@outlook.com
    • †Contact author: zxguo08@xjtu.edu.cn

    Phys. Rev. B 113, 125401 – Published 2 March, 2026

    DOI: https://doi.org/10.1103/dm4z-p9kt

    Abstract

    Anisotropic magnetoresistance (AMR) plays a critical role in spintronic memory and magnetic sensing devices. Although AMR is generally weak in bulk magnets, it is markedly enhanced in two-dimensional systems. However, its systematic evolution with dimensionality remains largely unexplored. Here we investigate the dimensional dependence of AMR in the van der Waals antiferromagnet MnBi2Te4 using density functional theory and Wannier-interpolated Boltzmann transport methods. Our results reveal a pronounced increase in the out-of-plane AMR as the sample thickness decreases, rising from 19.57% in the bulk to 42.93%, 52.17%, and 60.97% in the trilayer, bilayer, and monolayer, respectively. We uncover a mechanism governing this evolution: magnetization reorientation modulates the out-of-plane orbital hybridization between Bi and Te atoms, an effect that is strongly enhanced in thinner samples. This orbital hybridization variation directly tunes the spin-orbit coupling strength, leading to considerable band splitting that depends critically on the magnetization direction. Our work provides a unified microscopic understanding of dimension-dependent AMR and establishes MnBi2Te4 as a promising platform for designing tunable spintronic devices.

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