We propose a symmetry-resolved optical probe of intrinsic loop-current chirality in moiré materials, with twisted bilayer graphene as a representative realization. Interlayer interference generates chiral electronic circulation on triangular plaquettes, giving rise to an intrinsic geometric chirality that enters the second-order response through a $C_3$-selected angular harmonic of the Berry curvature and can be isolated by the orbital-angular-momentum difference $\mathrm{\Delta }\ell$ of interfering optical vortex beams. When moiré $C_3$ symmetry is preserved, the intrinsic contribution appears in the $\mathrm{\Delta }\ell =3$ channel of the helicity-dependent dc photocurrent, whereas $C_3$-breaking perturbations activate additional channels. These results establish angular-momentum-resolved nonlinear optics as a route to probing geometric chirality in moiré and other symmetry-engineered quantum materials.

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• Multiphoton or tunneling ionization & excitation
• Photocurrent
• Twistronics
• Graphene
• Moire materials
• Optical techniques