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    Critical phenomenon and two-dimensional Ising magnetic coupling in the chiral magnetic soliton host Mn1/3TaS2

    Jingjing Ma1,2,*, Fanying Meng2,*, Wei Liu3,†, Min Ge4,‡, Aina Wang5, Langsheng Ling1, Jiyu Fan6, Chunlan Ma7, Li Pi1,4 et al.

    Zhe Qu1 and Lei Zhang1,§

    • *These authors contributed equally to this work.
    • †Contact author: liuwei@ahu.edu.cn
    • ‡Contact author: gemin@ustc.edu.cn
    • §Contact author: zhanglei@hmfl.ac.cn

    Phys. Rev. B 112, 094439 – Published 19 September, 2025

    DOI: https://doi.org/10.1103/dkj8-1941

    Abstract

    The chiral magnetic soliton, a spiral localized spin texture with quantized topological charges, has garnered significant attention from both scientific and technological perspectives. The Mn-intercalated Mn1/3TaS2 hosts a one-dimensional topological chiral magnetic soliton. This work thoroughly investigates the critical phenomenon of Mn1/3TaS2 single crystals. Fitting the magnetic entropy change yields critical exponents of β=0.268±0.006, γ=1.392±0.008, and δ=6.209±0.007 with a critical temperature TC=70.12±0.01 K. Using these critical exponents, the magnetic entropy change curves are scaled into an independent universal curve, indicating the reliability and convergence of these parameters. The critical exponents of Mn1/3TaS2 are close to those of the two-dimensional (2D) Ising model characterized by a spatial and spin dimensionality of {d:n}={2:1}, which suggest strong anisotropic spin coupling in this system. Moreover, the spin interaction distance is estimated to decay as J(r)∼r−3.37(6). The H−T phase diagram for H⊥c is constructed, distinguishing the chiral magnetic helimagnetism (CHM), chiral soliton lattice (CSL), forced ferromagnetism (FFM), and paramagnetic (PM) phases. This clarification of the magnetic coupling and phase diagram enhances the understanding of chiral topological magnetism.

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