- Open Access
High-frequency susceptibility tensor in the inertial regime: Prediction for subterahertz magnonics in ferromagnets
Phys. Rev. B 112, 094433 – Published 17 September, 2025
DOI: https://doi.org/10.1103/dhk6-78tt
Abstract
Inertial spin dynamics alters the resonant spin wave excitation resulting in the modification of the resonance field and relaxation in microwave spectroscopy of ferromagnets described by the conventional Landau-Lifshitz-Gilbert (LLG) equation. Here we present a complete theoretical framework which quantitatively predicts the dynamic response of the magnetization for ferromagnetic systems exhibiting inertia. We compute the tensor of the high-frequency magnetic susceptibility analytically using the linearization of the inertial LLG equation, with fewer approximations than in the inertial Smit-Beljers approach. Our solution yields the precession (ferromagnetic resonance) and nutation resonance frequency, relaxation and intensity for an arbitrary free energy density, allowing straightforward quantitative analysis of inertial effects in magnetic resonances. Using the typical parameters of permalloy as an example we calculate the impact of materials parameters including Gilbert damping and inertial relaxation time on the conventional magnetic resonant response as well as the amplitude, linewidth, and frequency of the typically subterahertz nutation resonance.
Physics Subject Headings (PhySH)
Article Text
References (55)
- J. Gorchon, M. Hehn, G. Malinowski, and S. Mangin, Electronic transport induced ultrafast magnetization switching, J. Magn. Magn. Mater. 563, 169919 (2022).
- V. Baltz, A. Manchon, M. Tsoi, T. Moriyama, T. Ono, and Y. Tserkovnyak, Antiferromagnetic spintronics, Rev. Mod. Phys. 90, 015005 (2018).
- K. Olejník, T. Seifert, Z. Kašpar, V. Novák, P. Wadley, R. P. Campion, M. Baumgartner, P. Gambardella, P. Němec, J. Wunderlich et al., Terahertz electrical writing speed in an antiferromagnetic memory, Sci. Adv. 4, eaar3566 (2018).
- Y. Li, A.-L. Barra, S. Auffret, U. Ebels, and W. E. Bailey, Inertial terms to magnetization dynamics in ferromagnetic thin films, Phys. Rev. B 92, 140413(R) (2015).
- E. A. Gorbachev, L. A. Trusov, A. E. Sleptsova, E. S. Kozlyakova, L. N. Alyabyeva, S. R. Yegiyan, A. S. Prokhorov, V. A. Lebedev, I. V. Roslyakov, A. V. Vasiliev et al., Hexaferrite materials displaying ultra-high coercivity and sub-terahertz ferromagnetic resonance frequencies, Mater. Today 32, 13 (2020).
- M.-C. Ciornei, J. M. Rubí, and J.-E. Wegrowe, Magnetization dynamics in the inertial regime: Nutation predicted at short time scales, Phys. Rev. B 83, 020410(R) (2011).
- E. Olive, Y. Lansac, and J.-E. Wegrowe, Beyond ferromagnetic resonance: The inertial regime of the magnetization, Appl. Phys. Lett. 100, 192407 (2012).
- J.-E. Wegrowe and M.-C. Ciornei, Magnetization dynamics, gyromagnetic relation, and inertial effects, Am. J. Phys. 80, 607 (2012).
- M. Cherkasskii, M. Farle, and A. Semisalova, Nutation resonance in ferromagnets, Phys. Rev. B 102, 184432 (2020).
- R. Mondal, S. Großenbach, L. Rózsa, and U. Nowak, Nutation in antiferromagnetic resonance, Phys. Rev. B 103, 104404 (2021).
- S. V. Titov, W. J. Dowling, and Y. P. Kalmykov, Ferromagnetic and nutation resonance frequencies of nanomagnets with various magnetocrystalline anisotropies, J. Appl. Phys. 131, 193901 (2022).
- S. V. Titov, W. J. Dowling, V. A. Shchelkonogov, and A. S. Titov, Inertial rotational diffusion and magnetic relaxation of the spin system in a strong magnetic field, Phys. Rev. B 107, 174426 (2023).
- S. Ghosh, M. Cherkasskii, I. Barsukov, and R. Mondal, Theory of tensorial magnetic inertia in terahertz spin dynamics, Phys. Rev. B 110, 174430 (2024).
- C. S. Johnsen and A. Sudbø, Dynamically generated spin interactions and nutational spin inertia in normal metal–ferromagnet heterostructures, Phys. Rev. B 111, 144423 (2025).
- D. Angster, T. Dannegger, J. Schlegel, M. Evers, and U. Nowak, Nutational resonance modes in antiferromagnetic materials, Sci. Rep. 15, 21543 (2025).
- V. Unikandanunni, R. Medapalli, M. Asa, E. Albisetti, D. Petti, R. Bertacco, E. E. Fullerton, and S. Bonetti, Inertial spin dynamics in epitaxial cobalt films, Phys. Rev. Lett. 129, 237201 (2022).
- K. Neeraj, N. Awari, S. Kovalev, D. Polley, N. Zhou Hagström, S. S. P. K. Arekapudi, A. Semisalova, K. Lenz, B. Green, J.-C. Deinert et al., Inertial spin dynamics in ferromagnets, Nat. Phys. 17, 245 (2021).
- A. De, J. Schlegel, A. Lentfert, L. Scheuer, B. Stadtmüller, P. Pirro, G. von Freymann, U. Nowak, and M. Aeschlimann, Magnetic nutation: Transient separation of magnetization from its angular momentum, Phys. Rev. B 111, 014432 (2025).
- M. Cherkasskii, I. Barsukov, R. Mondal, M. Farle, and A. Semisalova, Theory of inertial spin dynamics in anisotropic ferromagnets, Phys. Rev. B 106, 054428 (2022).
- M. G. Quarenta, M. Tharmalingam, T. Ludwig, H. Y. Yuan, L. Karwacki, R. C. Verstraten, and R. A. Duine, Bath-induced spin inertia, Phys. Rev. Lett. 133, 136701 (2024).
- D. Thonig, O. Eriksson, and M. Pereiro, Magnetic moment of inertia within the torque-torque correlation model, Sci. Rep. 7, 931 (2017).
- S. Bhattacharjee, L. Nordström, and J. Fransson, Atomistic spin dynamic method with both damping and moment of inertia effects included from first principles, Phys. Rev. Lett. 108, 057204 (2012).
- R. Mondal, M. Berritta, A. K. Nandy, and P. M. Oppeneer, Relativistic theory of magnetic inertia in ultrafast spin dynamics, Phys. Rev. B 96, 024425 (2017).
- K. Neeraj, M. Pancaldi, V. Scalera, S. Perna, M. d'Aquino, C. Serpico, and S. Bonetti, Magnetization switching in the inertial regime, Phys. Rev. B 105, 054415 (2022).
- L. Winter, S. Großenbach, U. Nowak, and L. Rózsa, Nutational switching in ferromagnets and antiferromagnets, Phys. Rev. B 106, 214403 (2022).
- I. Makhfudz, Y. Hajati, and E. Olive, High-temperature magnetization reversal in the inertial regime, Phys. Rev. B 106, 134415 (2022).
- R. Mondal and A. Kamra, Spin pumping at terahertz nutation resonances, Phys. Rev. B 104, 214426 (2021).
- P.-B. He, Large-amplitude and widely tunable self-oscillations enabled by the inertial effect in uniaxial antiferromagnets driven by spin-orbit torques, Phys. Rev. B 108, 184418 (2023).
- R. Rodriguez, M. Cherkasskii, R. Jiang, R. Mondal, A. Etesamirad, A. Tossounian, B. A. Ivanov, and I. Barsukov, Spin inertia and auto-oscillations in ferromagnets, Phys. Rev. Lett. 132, 246701 (2024).
- R. Bastardis, F. Vernay, and H. Kachkachi, Magnetization nutation induced by surface effects in nanomagnets, Phys. Rev. B 98, 165444 (2018).
- M. P. Adams, R. Bastardis, A. Michels, and H. Kachkachi, Low-frequency signature of magnetization nutation in nanomagnets, Phys. Rev. B 110, 054415 (2024).
- I. Makhfudz, E. Olive, and S. Nicolis, Nutation wave as a platform for ultrafast spin dynamics in ferromagnets, Appl. Phys. Lett. 117, 132403 (2020).
- M. Cherkasskii, M. Farle, and A. Semisalova, Dispersion relation of nutation surface spin waves in ferromagnets, Phys. Rev. B 103, 174435 (2021).
- A. M. Lomonosov, V. V. Temnov, and J.-E. Wegrowe, Anatomy of inertial magnons in ferromagnetic nanostructures, Phys. Rev. B 104, 054425 (2021).
- S. V. Titov, W. J. Dowling, Y. P. Kalmykov, and M. Cherkasskii, Nutation spin waves in ferromagnets, Phys. Rev. B 105, 214414 (2022).
- R. Mondal and L. Rózsa, Inertial spin waves in ferromagnets and antiferromagnets, Phys. Rev. B 106, 134422 (2022).
- M. d'Aquino, S. Perna, M. Pancaldi, R. Hertel, S. Bonetti, and C. Serpico, Micromagnetic study of inertial spin waves in ferromagnetic nanodots, Phys. Rev. B 107, 144412 (2023).
- Z. Gareeva and K. Guslienko, Nutation excitations in the gyrotropic vortex dynamics in a circular magnetic nanodot, Nanomaterials 13, 461 (2023).
- G. Dieterle, J. Förster, H. Stoll, A. S. Semisalova, S. Finizio, A. Gangwar, M. Weigand, M. Noske, M. Fähnle, I. Bykova, J. Grafe, D. A. Bozhko, H. Y. Musiienko-Shmarova, V. Tiberkevich, A. N. Slavin, C. H. Back, J. Raabe, G. Schutz, and S. Wintz, Coherent excitation of heterosymmetric spin waves with ultrashort wavelengths, Phys. Rev. Lett. 122, 117202 (2019).
- S. Mayr, J. Förster, S. Finizio, K. Schultheiss, R. A. Gallardo, R. Narkovicz, G. Dieterle, A. Semisalova, J. Bailey, E. Kirk et al., Time-resolved x-ray imaging of nanoscale spin-wave dynamics at multi-GHz frequencies using low-alpha synchrotron operation, Appl. Phys. Rev. 11, 041411 (2024).
- E. Olive, Y. Lansac, M. Meyer, M. Hayoun, and J.-E. Wegrowe, Deviation from the Landau-Lifshitz-Gilbert equation in the inertial regime of the magnetization, J. Appl. Phys. 117, 213904 (2015).
- B. W. Zingsem, M. Winklhofer, R. Meckenstock, and M. Farle, Unified description of collective magnetic excitations, Phys. Rev. B 96, 224407 (2017).
- S. V. Vonsovskij and D. Ter Haar, Ferromagnetic Resonance : The Phenomenon of Resonant Absorption of a High-Frequency Magnetic Field in Ferromagnetic Substances, 1st ed., International series of monographs in solid state physics (Pergamon Press, Oxford, 1966).
- W. Frank and P. von Brentano, Classical analogy to quantum mechanical level repulsion, Am. J. Phys. 62, 706 (1994).
- L. Novotny, Strong coupling, energy splitting, and level crossings: A classical perspective, Am. J. Phys. 78, 1199 (2010).
- M. Farle, A. Berghaus, and K. Baberschke, Magnetic anisotropy of Gd (0001)/W (110) monolayers, Phys. Rev. B 39, 4838 (1989).
- M. Farle, Ferromagnetic resonance of ultrathin metallic layers, Rep. Prog. Phys. 61, 755 (1998).
- Y. Zhao, Q. Song, S.-H. Yang, T. Su, W. Yuan, S. S. Parkin, J. Shi, and W. Han, Experimental investigation of temperature-dependent Gilbert damping in permalloy thin films, Sci. Rep. 6, 22890 (2016).
- T. Strusch, K. Lenz, R. Meckenstock, R. Bali, J. Ehrler, J. Lindner, J. Fassbender, M. Farle, K. Potzger, and A. Semisalova, Spin pumping at interfaces with ferro-and paramagnetic films acting as spin source and spin sink, J. Appl. Phys. 132, 213906 (2022).
- E. Barati, M. Cinal, D. M. Edwards, and A. Umerski, Gilbert damping in magnetic layered systems, Phys. Rev. B 90, 014420 (2014).
- J. Wiemeler, A. C. Aktas, M. Farle, and A. Semisalova, Epitaxial Fe/Rh bilayers for efficient spin-to-charge conversion, Appl. Phys. Lett. 124, 212404 (2024).
- Y. Li, F. Zeng, S. S.-L. Zhang, H. Shin, H. Saglam, V. Karakas, O. Ozatay, J. E. Pearson, O. G. Heinonen, Y. Wu, A. Hoffmann, and W. Zhang, Giant anisotropy of Gilbert damping in epitaxial CoFe films, Phys. Rev. Lett. 122, 117203 (2019).
- Z. Lu, I. P. Miranda, S. Streib, Q. Xu, R. Cheenikundil, M. Pereiro, E. Sjöqvist, O. Eriksson, A. Bergman, D. Thonig, and A. Delin, Chemical disorder effects on Gilbert damping of FeCo alloys, Phys. Rev. B 110, 174428 (2024).
- C. Dubs, O. Surzhenko, R. Thomas, J. Osten, T. Schneider, K. Lenz, J. Grenzer, R. Hübner, and E. Wendler, Low damping and microstructural perfection of sub-40 nm-thin yttrium iron garnet films grown by liquid phase epitaxy, Phys. Rev. Mater. 4, 024416 (2020).
- M. C. Onbasli, A. Kehlberger, D. H. Kim, G. Jakob, M. Kläui, A. V. Chumak, B. Hillebrands, and C. A. Ross, Pulsed laser deposition of epitaxial yttrium iron garnet films with low Gilbert damping and bulk-like magnetization, APL Mater. 2, 106102 (2014).