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    Suppression of ferromagnetism and emergence of a cluster-glass state in Sr1−x(La0.5K0.5)xRuO3: Muon spin relaxation and neutron diffraction studies

    Ikuto Kawasaki1,*, Hideaki Ebisawa2, Nagisa Mitsugi2, Yuka Shiozawa2, Ryosuke Koizumi2, Kenji Ohoyama3,4, Kazuaki Iwasa3,4, Wataru Higemoto5, Jumpei G. Nakamura6 et al.

    James S. Lord7 and Makoto Yokoyama2,3

    • *Contact author: kawasaki.ikuto@jaea.go.jp

    Phys. Rev. B 114, 214404 – Published 6 October, 2026

    DOI: https://doi.org/10.1103/dckn-ytyv

    Abstract

    We have performed muon spin relaxation (μSR) and neutron powder diffraction experiments on the ferromagnet Sr1−x(La0.5K0.5)xRuO3. SrRuO3 shows a ferromagnetic (FM) order below 160 K, and the FM ordering temperature is monotonically suppressed as x increases, eventually vanishing at the critical concentration xc = 0.5. During this suppression process, the FM ordered state evolves into an FM cluster-glass state for x ≥ 0.4. Neutron scattering intensity due to the FM order develops below the magnetic ordering temperatures, but no antiferromagnetic peaks have been observed in either the FM or cluster-glass states within the experimental accuracy. The internal field at lowest temperatures revealed by the μSR experiments is monotonically suppressed as x increases. In contrast, the magnetic volume fraction Vf at lowest temperatures decreases only moderately with x up to x = 0.3, but drops rapidly near the critical concentration. The fact that Vf is less than 1 for x ≥ 0.3 is expected to be related to the origin of the cluster-glass state formation. We also found that the muon relaxation rate due to magnetic fluctuations in the cluster-glass state increases as x approaches xc, reflecting progressive destabilization of the cluster-glass state due to the reduction of Vf. These results indicate that the magnetically ordered states of Sr1−x(La0.5K0.5)xRuO3 are strongly affected by the disorder effect, and the suppression process of the FM order is largely different from that in a clean system. We compare the present experimental results with those for other Sr-site substituted systems, and discuss the differences in their magnetic properties and how they are affected by the disorder effect.

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