Export citation

Export citation

Choose format for download:

Download Citation
  • Letter

Static, dynamic, and tunneling fingerprints of antiferromagnetism in layered NiCl2

Liguo Zhang1,*,†, Shilin Li1,2,3,*, Yufeng Gao1,2,3,*, Junhai Ren1,‡, Qin Wang1, Dapeng Zhao1, Bo Bai4, Guangcun Shan5,6, and Katsumi Tanigaki1,§

  • *These authors contributed equally to this work.
  • †Contact author: zhanglg@baqis.ac.cn
  • ‡Contact author:renjh@baqis.ac.cn
  • §Contact author: katsumitanigaki@baqis.ac.cn

Phys. Rev. B 113, L100402 – Published 5 March, 2026

DOI: https://doi.org/10.1103/d73h-v5p8

Abstract

The recent surge of interest in magnetism in van der Waals (vdW) crystals has opened opportunities for exploring antiferromagnetic order and spin dynamics in the two-dimensional limit. Here, we present a comprehensive study of the layered antiferromagnetic NiCl2, combining static magnetization, broadband microwave absorption spectroscopy, and tunneling transport measurements. Despite early studies of bulk NiCl2, our systematic approach provides a modern reexamination of its magnetic properties with several new insights. We find nearly identical in-plane and out-of-plane saturation fields once demagnetization corrections are applied, as well as a pronounced spin-flop transition at low fields. The Néel transition temperature (TN) shows minimal anisotropy at low fields but undergoes a distinct crossover between in-plane and out-of-plane field orientations at high fields. Spin resonance experiments reveal strongly anisotropic behavior: robust in-plane antiferromagnetic resonance modes are observed over a broad gigahertz frequency and temperature range, while out-of-plane measurements show suppressed response near TN. This enables the extraction of the effective g factor across a wide temperature window. Furthermore, tunneling magnetoconductance through a thin NiCl2 flake barrier exhibits field-enhanced transmission with clear signatures of the spin-flop and saturation fields. Our findings establish NiCl2 as a model vdW antiferromagnet for studying the interplay of static order, spin dynamics, and tunneling transport, highlighting its potential for future applications in two-dimensional spintronics.

Physics Subject Headings (PhySH)

Authorization Required

We need you to provide your credentials before accessing this content.

Supplemental Material (Subscription Required)

References (Subscription Required)

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation