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    Observation of the surface hybridization gap in the electrical transport properties of the ultrathin topological insulator (Bi1−xSbx)2Te3

    Feike van Veen1,*, Sofie Kölling1,*, Stijn R. de Wit1, Roel Metsch1, Daniel Rosenbach2, Chuan Li1, and Alexander Brinkman1

    • *These authors contributed equally to this work.

    Phys. Rev. B 112, 045425 – Published 23 July, 2025

    DOI: https://doi.org/10.1103/d5xc-bvmx

    Abstract

    We study the three-dimensional topological insulator (Bi1−xSbx)2Te3 in its ultrathin limit, i.e., when the thickness is of the same order as the surface-state penetration depth. It is expected that in this limit a hybridization gap opens at the Dirac point, which gives rise to a quantum spin Hall (QSH) or insulating phase, depending on the material thickness. We fabricate (Bi1−xSbx)2Te3 Hall bars with a thicknesses of 6 and 9 nm and measure an insulating phase around the Dirac point for low bias and at sub-Kelvin temperatures only in samples fabricated from the 6 nm films, which indicates the presence of a hybridization gap. The effect of a perpendicular magnetic field on the hybridization gap is studied but remains partially unresolved. The results form an important step towards experimentally realizing the quantum spin Hall state via hybridization in ultrathin films of (Bi1−xSbx)2Te3, yet, they also expose a knowledge gap regarding transport measurements in these systems.

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