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    Anomalous Hall effect and topological Hall effect in the centrosymmetric antiferromagnet V1/4NbSe2

    Kun Han1,2,*, Xiao-Ping Ma3,*, Huan Wang1,2,4, Jun-Fa Lin1,2, Yi-Ting Wang1,2, Xue Dong1,2, Yu Zhang1,2, Huai-Xin Yang3,5, and Tian-Long Xia1,2,6,7,†

    • *These authors contributed equally to this work.
    • †Contact author: tlxia@ruc.edu.cn

    Phys. Rev. B 113, 094455 – Published 30 March, 2026

    DOI: https://doi.org/10.1103/ck1l-fl82

    Abstract

    The pursuit of high-speed, low-power spintronic devices has driven extensive research into the anomalous Hall effect (AHE) in antiferromagnets. Concurrently, the topological Hall effect (THE), a hallmark of chiral spin textures, has emerged as a critical probe of nontrivial magnetism. Here, we report the synthesis and physical properties of V1/4NbSe2, a centrosymmetric van der Waals antiferromagnet with a 2×2 superlattice structure. It exhibits two successive antiferromagnetic (AFM) transitions: a paramagnetic-to-AFM1 transition at TN = 14.7 K, followed by an AFM1-to-AFM2 transition below Tt≈ 6.4 K. Magnetic characterization reveals dominant AFM interactions, weak magnetocrystalline anisotropy, and nonlinear magnetization suggestive of a spin-flop-like transition. Electrical transport demonstrates coexisting AHE and THE phenomena. The AHE, which is likely dominated by the intrinsic mechanism, peaks near TN with a conductivity of ∼160 Ω−1cm−1. Notably, the THE emerges exclusively within the AFM2 phase, suggesting its origin of a field-induced nonzero scalar spin chirality. Magnetoresistance exhibits butterfly-shaped hysteresis loops stemming from spin-dependent electron scattering. These phenomena collectively point to an intricate magnetic ground state in the absence of Dzyaloshinskii-Moriya interaction, warranting further investigation to unravel the underlying spin configuration.

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