Anomalous Hall effect and topological Hall effect in the centrosymmetric antiferromagnet
Phys. Rev. B 113, 094455 – Published 30 March, 2026
DOI: https://doi.org/10.1103/ck1l-fl82
Abstract
The pursuit of high-speed, low-power spintronic devices has driven extensive research into the anomalous Hall effect (AHE) in antiferromagnets. Concurrently, the topological Hall effect (THE), a hallmark of chiral spin textures, has emerged as a critical probe of nontrivial magnetism. Here, we report the synthesis and physical properties of , a centrosymmetric van der Waals antiferromagnet with a superlattice structure. It exhibits two successive antiferromagnetic (AFM) transitions: a paramagnetic-to-AFM1 transition at = 14.7 K, followed by an AFM1-to-AFM2 transition below 6.4 K. Magnetic characterization reveals dominant AFM interactions, weak magnetocrystalline anisotropy, and nonlinear magnetization suggestive of a spin-flop-like transition. Electrical transport demonstrates coexisting AHE and THE phenomena. The AHE, which is likely dominated by the intrinsic mechanism, peaks near with a conductivity of . Notably, the THE emerges exclusively within the AFM2 phase, suggesting its origin of a field-induced nonzero scalar spin chirality. Magnetoresistance exhibits butterfly-shaped hysteresis loops stemming from spin-dependent electron scattering. These phenomena collectively point to an intricate magnetic ground state in the absence of Dzyaloshinskii-Moriya interaction, warranting further investigation to unravel the underlying spin configuration.