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Magnetoelastic mapping of the high-field phase diagram in the topological cubic helimagnet SrFeO3

Masaki Gen1,2,*, Shun Okumura2,3,4,†, Shusaku Imajo1,5, Taro Nakajima1,2,6, Karel Prokes7, Shunsuke Kitou5, Yusuke Tokunaga5, Yoichi Nii8, Koichi Kindo1 et al.

Yoshimitsu Kohama1, Shintaro Ishiwata9, and Taka-hisa Arima2,5

  • *Contact author: gen@issp.u-tokyo.ac.jp
  • †Contact author: okumura@ap.t.u-tokyo.ac.jp

Phys. Rev. B 114, 264406 – Published 4 November, 2026

DOI: https://doi.org/10.1103/ch1m-ppsm

Abstract

The cubic perovskite SrFeO3 is a prototypical centrosymmetric itinerant magnet that hosts a quadruple-Q hedgehog-antihedgehog lattice and exhibits a complex magnetic-field–temperature phase diagram. Yet, the microscopic mechanism underlying the emergence of its versatile multiple-Q phases remains unresolved. Here, we reveal the field-orientation dependence of the magnetic phase diagram and establish an effective spin Hamiltonian for SrFeO3 that incorporates a cubic single-ion anisotropy together with bilinear and biquadratic interactions in momentum space, which originate from the spin-charge coupling. In addition, we observe magnetoelastic signatures of a redistribution of the ligand-hole density upon entering the forced ferromagnetic phase. These findings are consistent with an important role of electronic itinerancy associated with the formation of a ligand-hole band in stabilizing multiple-Q phases.

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