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Magnetoelastic mapping of the high-field phase diagram in the topological cubic helimagnet
Phys. Rev. B 114, 264406 – Published 4 November, 2026
DOI: https://doi.org/10.1103/ch1m-ppsm
Abstract
The cubic perovskite is a prototypical centrosymmetric itinerant magnet that hosts a quadruple- hedgehog-antihedgehog lattice and exhibits a complex magnetic-field–temperature phase diagram. Yet, the microscopic mechanism underlying the emergence of its versatile multiple- phases remains unresolved. Here, we reveal the field-orientation dependence of the magnetic phase diagram and establish an effective spin Hamiltonian for that incorporates a cubic single-ion anisotropy together with bilinear and biquadratic interactions in momentum space, which originate from the spin-charge coupling. In addition, we observe magnetoelastic signatures of a redistribution of the ligand-hole density upon entering the forced ferromagnetic phase. These findings are consistent with an important role of electronic itinerancy associated with the formation of a ligand-hole band in stabilizing multiple- phases.