L-point quadrupole order under magnetic field in cubic
Phys. Rev. B 113, 165138 – Published 20 April, 2026
DOI: https://doi.org/10.1103/cflz-9y82
Abstract
We study quadrupole orders in heavy-fermion compound under magnetic fields on the basis of the Landau theory. Assuming electric quadrupolar orders in the cubic symmetry with the ordering wave number at the L points in the face-centered-cubic lattice Brillouin zone as observed experimentally, we construct a Landau free energy and analyze the resulting free energy. We find that the unidentified high-temperature ordered phase under the magnetic field reported earlier arises from the rotation of the quadrupole moments of electrons on the Pr site. We also discuss the phase diagram for other magnetic-field directions and possible double- quadrupolar orders in this system.