Phase diagram and spin dynamics of the spin- bilinear-biquadratic-bicubic Heisenberg model on the square lattice
Phys. Rev. B 113, 155111 – Published 6 April, 2026
DOI: https://doi.org/10.1103/ccyk-yzqm
Abstract
Multipolar interactions play a pivotal role in governing emergent phenomena in quantum materials, including multiferroics and quantum magnetism. In this work, we determine the ground-state phase diagram of the nearest-neighbor spin- bilinear-biquadratic-bicubic Heisenberg model on the square lattice through a combination of mean-field theory and exact diagonalization. We demonstrate that quantum fluctuations can drive the emergence of multisublattice ordered phases, even on a bipartite lattice, provided that multipolar interactions are sufficiently strong. To characterize the excitation spectra across these distinct phases, we develop cluster spin-wave theory—an extension of conventional linear spin-wave theory—which enables the reliable description of both low-energy magnon dispersions and high-energy multimagnon continua. Our findings offer valuable insights into the nature of collective excitations in strongly correlated spin systems and establish a robust theoretical framework for understanding spin dynamics in complex quantum magnets.