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    Coexistence of mixed-dimensional fluctuations and incommensurate long-range order in the frustrated antiferromagnet Ce5AgPb3

    Zhijie Ma1,2, Ying Sun1,*, Jiechen Luo1, Sihao Deng3,4,†, Hongde Wang3,5, Xiuliang Yuan2, Kaiqi Zhang1, Lunhua He2,3,6, Cong Wang5,7 et al.

    Youguo Shi2,6,‡

    • *Contact author: sunying@buaa.edu.cn
    • †Contact author: dengsh@ihep.ac.cn
    • ‡Contact author: ygshi@iphy.ac.cn

    Phys. Rev. B 114, 024406 – Published 6 July, 2026

    DOI: https://doi.org/10.1103/ccgc-z6gx

    Abstract

    Low-dimensional systems host exotic quantum phenomena arising from dimensional confinement and strong electron correlations. Here, we report a prototypical case of site-specific mixed dimensionality in Ce5AgPb3, which originates from inequivalent Ce1(6g) and Ce2(4d) sites. The frustrated quasi-two-dimensional Ce1 sublattice develops an incommensurate noncollinear antiferromagnetic order with moment modulation characterized by a propagation vector of kz≈0.84 below TN=10K, exhibiting two-dimensional Ising critical behavior [β=0.123(6)]. The quasi-one-dimensional Ce2 chains remain magnetically disordered but host dynamic spin fluctuations decoupled from long-range magnetic order, revealed by a persistent −H2-dependent component in negative magnetoresistance. The coexistence of long-range order and mixed-dimensional fluctuations drives the formation of a strongly correlated electronic state with a large γ of 345.6mJmol−1K−2. Our work thus provides a unique, site-specific paradigm for disentangling the complex magnetism in bulk materials with mixed-dimensional motifs.

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