Doping-tuned magnetic anisotropy and anomalous Hall conductivity in the van der Waals room-temperature ferromagnet
Phys. Rev. B 113, 064435 – Published 24 February, 2026
DOI: https://doi.org/10.1103/bk11-6yym
Abstract
High-temperature ferromagnetism and large anomalous Hall conductivity (AHC) in two-dimensional (2D) magnets are highly desirable for ultrathin 2D spintronic devices, as they endow these devices with superior magnetic stability and efficient spin-current conversion capabilities, thereby driving advancements in low-power and high-density spintronic technologies. Here, by first-principles calculations, we study the electronic and magnetic properties of which is an energetically and dynamically stable van der Waals ferromagnet with an in-plane magnetic anisotropy. Notably, we show that the Curie temperatures of monolayer, bilayer, triple-layer, quadruple-layer, and bulk are all above room temperature. By reorienting their spins from in-plane to out-of-plane, monolayer, few-layer, and bulk exhibit a large AHC range from 427–540 S/cm at the Fermi level, which is related to the mirror symmetry breaking. Furthermore, monolayer display perpendicular magnetic anisotropy under electron doping and retains the high Curie temperature and large AHC. Our findings suggest that van der Waals room-temperature ferromagnet holds promising applications in practical spintronic devices.