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Universal route to chiral Ising superconductivity in monolayer TaS2 and NbSe2

Lucia Gibelli1, Simon Höcherl1, Julian Siegl1, Viliam Vaňo2, Somesh C. Ganguli2, Magdalena Marganska3, and Milena Grifoni1,*

  • *Contact author: Milena.Grifoni@ur.de

Phys. Rev. B 112, L220505 – Published 29 December, 2025

DOI: https://doi.org/10.1103/bh1n-sc95

Abstract

We investigate Ising superconductivity in two archetypal intrinsic superconductors, monolayer 1H−TaS2 and 1H−NbSe2, in a bottom-up approach. Using ab initio-based tight-binding parametrizations for the relevant low-energy d bands, the screened interaction is evaluated microscopically in a scheme including Bloch overlaps. In direct space, the screened potential for both systems displays long-range Friedel oscillations alternating in sign. Upon scaling, the oscillation pattern becomes universal, with the location of minima and maxima locked to the lattice. Solving the momentum-resolved gap equations, a chiral ground state with p-like symmetry is generically found. Due to the larger Ising spin-orbit coupling, the chiral gap is more anisotropic in TaS2 than in NbSe2. This is reflected in tunneling spectra displaying V-shaped features for the former, in quantitative agreement with low-temperature scanning tunneling experiments on TaS2. At the same time, our results reconcile the apparent discordance with hard gap tunneling spectra reported for the sibling NbSe2.

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