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Uniform electronic states and s-wave superconductivity in a strongly disordered high-entropy compound X0.6Pt0.4Sb (X = Ru, Rh, Pd, Ir)

Yufu Yamada1, Shunsaku Kitagawa1,*, Taishi Ihara1, Kenji Ishida1, Naoto Uematsu2, Daigorou Hirai2, and Koshi Takenaka2

  • *Contact author: kitagawa.shunsaku.8u@kyoto-u.ac.jp

Phys. Rev. B 112, L020508 – Published 31 July, 2025

DOI: https://doi.org/10.1103/b4nw-c4zy

Abstract

High-entropy compounds, where multiple elements occupy a single crystallographic site in a highly disordered manner, challenge conventional understandings of electronic structures based on periodicity and well-defined band dispersion. Here, we report a detailed nuclear magnetic resonance study of the high-entropy superconductor X0.6Pt0.4Sb (X = Ru, Rh, Pd, Ir), revealing a spatially homogeneous electronic environment in the normal state, in stark contrast to its crystallographically disordered lattice. The superconducting state exhibits a small but solid Hebel-Slichter coherence peak followed by a significant decrease in the nuclear spin-lattice relaxation rate, providing compelling evidence for fully gapped s-wave pairing. Our findings not only deepen the understanding of superconductivity in highly disordered quantum materials but also open an alternative pathway for exploring superconducting states in entropy-stabilized systems.

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