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    Ferromagnetic transition in dilute Pd-Fe alloys

    C. Büscher, T. Auerswald, E. Scheer, A. Schröder, and H. v. Löhneysen

    H. Claus

    • Physikalisches Institut, Universität Karlsruhe, 7500 Karlsruhe, Germany

    • Kernforschungszentrum Karlsruhe, Institut für Technische Physik, Postfach 3640, 7500 Karlsruhe, Germany
    • Physikalisches Institut, Universität Karlsrhue, 7500 Karlsruhe, Germany

    Phys. Rev. B 46, 983 – Published 1 July, 1992

    DOI: https://doi.org/10.1103/PhysRevB.46.983

    Abstract

    We present low-field magnetization and specific-heat data for Pd1−xFex alloys, with x ranging from 0.08 to 0.6 at. % Fe. Both types of measurements were done on the same samples. The samples are more homogeneous than those used in previous investigations. We find that in contrast to previous suggestions, all samples undergo sharp ferromagnetic transitions with TC ranging from 0.4 K for the 0.08-at. % Fe alloy to 18.0 K for the 0.6-at. % Fe alloy. The specific-heat anomalies associated with the transitions have the form of a cusp very close to TC as determined from the magnetization. However, because of large fluctuations, these anomalies are very broad, extending to a region of temperatures well above TC. Combining our results with earlier data, we argue that the critical concentration for ferromagnetism in Pd-Fe alloys is near 0.01 at. % Fe, lower by a factor of 10 than previously assumed.

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