Export citation

Export citation

Choose format for download:

Download Citation

    Excitons and polaritons in monomolecular layers

    Michael R. Philpott

    Peter G. Sherman

    • IBM Research Laboratory, San Jose, California 95193

    • Institute of Theoretical Science and Department of Chemistry, University of Oregon, Eugene, Oregon 97403

    Phys. Rev. B 12, 5381 – Published 15 December, 1975

    DOI: https://doi.org/10.1103/PhysRevB.12.5381

    Abstract

    A theory of the coupling of photons to the exciton states of a monomolecular layer is presented. It is shown that the collective excitations (polaritons) of the layer are of mixed exciton-photon character. For transitions polarized perpendicular to the exciton wave vector there are two polariton branches, one is superradiant with radiative lifetimes (λa)2≃104 times shorter than for the free molecule, and the other does not radiate at all. This subradiant branch is defined for all frequencies ω below the molecular transition frequency ω0 and for ω≪ω0 corresponds to an electromagnetic wave trapped on the monolayer. The properties of polaritons on monolayers near the plane interface of two media are considered and the polariton dispersion relation examined for some special cases.

    Authorization Required

    We need you to provide your credentials before accessing this content.

    References (Subscription Required)

    Outline

    Information

    Sign In to Your Journals Account

    Filter

    Filter

    Article Lookup

    Enter a citation