- Letter
Exotic magnetic phase diagram and extremely robust antiferromagnetism in
Phys. Rev. B 111, L201110 – Published 13 May, 2025
DOI: https://doi.org/10.1103/PhysRevB.111.L201110
Abstract
The antiferromagnetic heavy-fermion compound belongs to the same family and bears similarities with the well-studied prototypical material , which demonstrates a unique behavior under applied magnetic field. Here, we report specific-heat measurements on a high-quality single crystal of in magnetic fields up to 35 T applied along both principal crystallographic directions. When the magnetic field is applied along the axis of the tetragonal crystal structure, two additional field-induced antiferromagnetic phases are observed, in agreement with previous reports. One of them is confined in a small area of the field-temperature phase diagram. The other one, which develops above T, is very robust against the field. Its transition temperature increases with field, reaches a maximum at T, and then starts to decrease. However, it tends to saturate towards the highest field of our measurements. For a field applied along the axis, the Néel temperature initially decreases with field, as expected for a typical antiferromagnet. Surprisingly, an additional phase emerges above T. It is most likely to be of the same origin as its counterpart observed above 2.5 T for the other field orientation. This phase is also unusually robust: Its transition temperature increases all the way up to 35 T, where it exceeds the zero field K. Finally, for both field directions, the phase diagrams contain rarely observed tricritical points of second-order phase transitions.