We demonstrate that, contrary to common wisdom, genuine multipartite entanglement (GME) can be abundantly generated from simple noncorrelated many-electron states. We show that the extracted GME can be maximized via spin-independent transformations derived from the quantum Fourier transform. We further demonstrate the possibility of maximizing the GME through localized orbitals in a variety of realistic systems and correlated states. Towards the exploitation of potentially useful entanglement, we rationalize system-specific and universal features of the extracted GME.

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• Electronic structure of atoms & molecules
• First-principles calculations
• Quantum correlations in quantum information
• 0-dimensional systems
• Electron techniques
• Quantum chemistry methods