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  • Letter

Constraints on the orbital flux phase in AV3Sb5 from the polar Kerr effect

Hao-Tian Liu1,2,3, Junkang Huang4, Tao Zhou4, and Wen Huang1,5,6,*

  • 1Shenzhen Institute for Quantum Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, Guangdong, China
  • 2Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China
  • 3University of Chinese Academy of Sciences, Beijing 100049, China
  • 4Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials, School of Physics, Guangdong-Hong Kong Joint Laboratory of Quantum Matter, and Frontier Research Institute for Physics, South China Normal University, Guangzhou 510006, China
  • 5International Quantum Academy, Shenzhen 518048, China
  • 6Guangdong Provincial Key Laboratory of Quantum Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China

  • *Contact author: huangw3@sustech.edu.cn

Phys. Rev. B 111, L041109 – Published 16 January, 2025

DOI: https://doi.org/10.1103/PhysRevB.111.L041109

Abstract

The AV3Sb5 (A= K, Rb, Cs) family of kagome metals hosts unconventional charge density wave (CDW) order whose nature is still an open puzzle. Accumulated evidences point to a time-reversal symmetry breaking (TRSB) orbital flux phase that carries loop currents. Such an order may support anomalous Hall effect. However, the polar Kerr effect measurements that probe the ac anomalous Hall conductivity seem to have yielded contradictory results. We first argue on symmetry grounds that some previously proposed orbital flux order, most notably the one with Star-of-David distortion, shall not give rise to anomalous Hall or polar Kerr effects. We further take the trihexagonal orbital flux phase as an exemplary kagome flux order that does exhibit anomalous Hall response and show that the Kerr rotation angle at two relevant experimental optical frequencies generally reaches microradians to sub-milliradians levels. A particularly sharp resonance enhancement is observed at around ℏω=1 eV, suggesting exceedingly large Kerr rotation at the corresponding probing frequencies not yet accessed by previous experiments. Our study provides important guidance to the interpretation of Kerr measurements on the CDW phase of AV3Sb5. In particular, we highlight the important fact that absence of Kerr signal cannot be equated with the absence of TRSB CDW order in AV3Sb5.

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