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Magnetization reversal of a ferromagnetic Pt/Co/Pt film by helicity dependent absorption of visible to near-infrared laser pulses

Kihiro T. Yamada1,2,*,†, Carl S. Davies1,3,*,‡, Fuyuki Ando4, Tian Li4, Teruo Ono4,5,6, Theo Rasing1, Alexey V. Kimel1, and Andrei Kirilyuk1,3

  • 1Radboud University, Institute for Molecules and Materials, Nijmegen 6525 AJ, The Netherlands
  • 2Department of Physics, Institute of Science Tokyo, Tokyo 152-8551, Japan
  • 3FELIX Laboratory, Radboud University, Toernooiveld 7, Nijmegen 6525 ED, The Netherlands
  • 4Institute for Chemical Research, Kyoto University, Uji 611-0011, Japan
  • 5Center for Spintronics Research Network, Institute for Chemical Research, Kyoto University, Uji, 611-0011, Japan
  • 6Center for Spintronics Research Network (CSRN), Graduate School of Engineering Science, Osaka University, Toyonaka 560-8531, Japan

  • *These authors contributed equally.
  • †Contact author: yamada@phys.sci.isct.ac.jp
  • ‡Contact author: c.davies@science.ru.nl

Phys. Rev. B 111, L020406 – Published 15 January, 2025

DOI: https://doi.org/10.1103/PhysRevB.111.L020406

Abstract

The practical difficulty in distinguishing the impact of magnetic circular dichroism and the inverse Faraday effect fuels intense debates over which mechanism predominantly drives the process of helicity dependent all-optical switching of magnetization in ferromagnets. Here, we quantitatively measure the efficiency of the switching process in a Pt/Co/Pt multilayer stack using visible- to near-infrared optical pulses. We find that the switching efficiency increases by a factor of 8.6 upon increasing the pumping wavelength from 0.5 to 1.1 μm, becoming 100% efficient at even longer wavelengths up to 2.0 μm. Our experimental results can be successfully explained by the phenomenon of magnetic circular dichroism, making a significant step towards resolving the long-standing controversy over the origin of the all-optical process of magnetization reversal in ferromagnets.

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