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  • Letter

Intermediate field-induced phase of the honeycomb magnet BaCo2(AsO4)2

Prashanta K. Mukharjee1,*, Bin Shen1, Sebastian Erdmann1, Anton Jesche1, Julian Kaiser1, Priya R. Baral2, Oksana Zaharko2, Philipp Gegenwart1,†, and Alexander A. Tsirlin3,‡

  • 1Experimental Physics VI, Center for Electronic Correlations and Magnetism, Institute of Physics, University of Augsburg, 86159 Augsburg, Germany
  • 2Laboratory for Neutron Scattering and Imaging (LNS), Paul Scherrer Institute (PSI), CH-5232 Villigen, Switzerland
  • 3Felix Bloch Institute for Solid-State Physics, University of Leipzig, 04103 Leipzig, Germany

  • *Contact author: pkmukharjee92@gmail.com
  • †Contact author: philipp.gegenwart@physik.uni-augsburg.de
  • ‡Contact author: altsirlin@gmail.com

Phys. Rev. B 110, L140407 – Published 21 October, 2024

DOI: https://doi.org/10.1103/PhysRevB.110.L140407

Abstract

We use magnetometry, calorimetry, and high-resolution capacitive dilatometry, as well as single-crystal neutron diffraction to explore the temperature-field phase diagram of the anisotropic honeycomb magnet BaCo2(AsO4)2. Our data reveal four distinct ordered states observed for in-plane magnetic fields. Of particular interest is the narrow region between 0.51 and 0.54 T that separates the up-up-down order from the fully polarized state and coincides with the field range where signatures of the spin-liquid behavior have been reported. We show that magnetic Bragg peaks persist in this intermediate phase, thus ruling out its spin-liquid nature. However, the simultaneous nonmonotonic evolution of nuclear Bragg peaks suggests the involvement of the lattice, witnessed also in other regions of the phase diagram where large changes in the sample length are observed upon entering the magnetically ordered states. Our data highlight the importance of lattice effects in BaCo2(AsO4)2.

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