- Letter
Frustrated Ising charge correlations in the kagome metal
Phys. Rev. B 110, L140304 – Published 15 October, 2024
DOI: https://doi.org/10.1103/PhysRevB.110.L140304
Abstract
Here we resolve the real-space nature of the high-temperature, short-range charge correlations in the kagome metal . Diffuse scattering appears along a frustrated wave vector at temperatures far exceeding the charge order transition K, preempting long-range charge order with wave vectors along . Using a combination of real space and reciprocal space analysis, we resolve the nature of the interactions between the primary out-of-plane Sc-Sn chain instability and the secondary strain-mediated distortion of the in-plane V kagome network. A minimal model of the diffuse scattering data reveals a high-temperature, short-ranged “zig-zag” phase of in-plane correlations that maps to a frustrated triangular lattice Ising model with antiferromagnetic interactions and provides a real-space understanding of the origin of frustrated charge order in this material.