- Letter
Nonanalytic magnetic response and intrinsic ferromagnetic clusters in a kagome spin-liquid candidate
Phys. Rev. B 110, L121105 – Published 11 September, 2024
DOI: https://doi.org/10.1103/PhysRevB.110.L121105
Abstract
Finding distinct signatures of a quantum spin liquid (QSL) is an ongoing quest in condensed matter physics, invariably complicated by the presence of disorder in real materials. In this regard the two-dimensional kagome system , where the vast mismatch in size of Y and Cu avoids substitutional disorder, otherwise present in kagome materials, has emerged as a favorable candidate. In crystals of this system, with and no long-range order, we report an unusual field-dependent magnetization , where changes linearly with , the absolute value of the field, in contrast to the expected quadratic behavior. Model calculations with a distribution of ferromagnetic (FM) clusters faithfully capture the observed features. YCOB-Cl exhibits a field-enhanced heat capacity expected in certain spin-liquid models. However, a concomitant linear behavior in the spin susceptibility has been lacking. Our work suggests that FM clusters, by dominating the contribution to the susceptibility, mask the true underlying behavior.