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Determination of the Néel vector in rutile altermagnets through x-ray magnetic circular dichroism: The case of MnF2

A. Hariki1, T. Okauchi1, Y. Takahashi1, and J. Kuneš2

  • 1Department of Physics and Electronics, Graduate School of Engineering, Osaka Metropolitan University, 1-1 Gakuen-cho, Nakaku, Sakai, Osaka 599-8531, Japan
  • 2Department of Condensed Matter Physics, Faculty of Science, Masaryk University, Kotlářská 2, 611 37 Brno, Czechia

Phys. Rev. B 110, L100402 – Published 5 September, 2024

DOI: https://doi.org/10.1103/PhysRevB.110.L100402

Abstract

We present a numerical simulation of x-ray magnetic circular dichroism (XMCD) at the L2,3 edge of Mn in a representative rutile altermagnet MnF2 using a combination of density functional theory plus exact diagonalization of the atomic model. We explore how the dichroic spectra vary with the orientation of the light propagation vector and the Néel vector. An exact relationship between the XMCD spectra for different orientations of the Néel vector, valid in the absence of the valence spin-orbit coupling and core-valence multipole interaction, is derived and its approximate validity for the full Hamiltonian verified by numerical calculation. This relationship allows one to determine the in-plane orientation of the Néel vector using the XMCD spectra alone.

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