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Phonon thermal Hall effect in nonmagnetic Y2Ti2O7

Rohit Sharma1,*, Martin Valldor1,2, and Thomas Lorenz1,†

  • 1II. Physikalisches Institut, Universität zu Köln, Zülpicher Strasse 77, 50937 Köln, Germany
  • 2Centre for Materials Science and Nanotechnology (SMN), Department of Chemistry, University of Oslo, Oslo N-0371, Norway

  • *Contact author: sharma@ph2.uni-koeln.de
  • †Contact author: tl@ph2.uni-koeln.de

Phys. Rev. B 110, L100301 – Published 3 September, 2024

DOI: https://doi.org/10.1103/PhysRevB.110.L100301

Abstract

We report an investigation of the phonon thermal Hall effect in single crystal samples of Y2Ti2O7, Dy2Ti2O7, and DyYTi2O7. We measured the field-linear thermal Hall effect in all three samples. The temperature dependence of thermal Hall conductivities shows a peak around 15 K, which coincides with the peak positions of the longitudinal thermal conductivities. The temperature-dependent longitudinal thermal conductivities indicates that phonons dominate thermal transport in all three samples. However, the presence of Dy3+ magnetic ions introduces significant effects on the field dependence of the longitudinal thermal conductivities. The thermal Hall ratio is sizable in all three samples and consistent with the values reported for other insulating materials exhibiting a phononic thermal Hall effect, though their exact underlying mechanism remains yet to be identified. The thermal Hall ratio is nearly the same for Y2Ti2O7 and DyYTi2O7, and slightly larger for Dy2Ti2O7, suggesting that magnetic impurities are less significant in generating the phononic thermal Hall effect. Our observations of the phononic thermal Hall effect support an intrinsic origin in Y2Ti2O7 and suggest a combination of intrinsic and extrinsic effects in Dy2Ti2O7 and DyYTi2O7.

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