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  • Letter

Magnetic field induced critical dynamics in magnetoelectric TbPO4

Ch. P. Grams, M. Grüninger, and J. Hemberger*

  • *Contact author: hemberger@ph2.uni-koeln.de

Phys. Rev. B 110, L041106 – Published 1 July, 2024

DOI: https://doi.org/10.1103/PhysRevB.110.L041106

Abstract

We report on the magnetoelectric dynamics in the linear magnetoelectric antiferromagnet TbPO4 studied by broadband dielectric spectroscopy. For the phase transition into the magnetoelectric antiferromagnetic phase at TN≈2.3K, a finite magnetic field H induces critical behavior in the quasistatic permittivity ɛ′(T). Plotting the corresponding anomaly as a function of T/TN(H), we observe the scaling behavior Δɛ′∝H2, a clear fingerprint of linear magnetoelectric antiferromagnets. Above the phase transition, we find a critical slowing down of the ferroic fluctuations in finite magnetic field. This behavior can be understood via a magnetic field induced relaxational response that resembles the soft-mode behavior in canonical ferroelectrics and multiferroics.

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