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  • Letter

Emergence of radial Rashba spin-orbit fields in twisted van der Waals heterostructures

Tobias Frank, Paulo E. Faria Junior*, Klaus Zollner, and Jaroslav Fabian

  • *Contact author: fariajunior.pe@gmail.com

Phys. Rev. B 109, L241403 – Published 12 June, 2024

DOI: https://doi.org/10.1103/PhysRevB.109.L241403

Abstract

Rashba spin-orbit coupling is a quintessential spin interaction appearing in virtually any electronic heterostructure. Its paradigmatic spin texture in the momentum space forms a tangential vector field. Using first-principles investigations, we demonstrate that in twisted homobilayers and heteromultilayers, the Rashba spin texture can be predominantly radial, parallel to the momentum. Specifically, we study four experimentally relevant structures: twisted bilayer graphene (Gr), twisted bilayer WSe2, and twisted multilayers WSe2/Gr/WSe2 and WSe2/Gr/Gr/WSe2. We show that the Rashba spin texture in such structures can be controlled by an electric field, allowing to tune it from radial to tangential. Such spin-orbit engineering should be useful for designing spin-charge conversion and spin-orbit torque schemes, as well as for controlling correlated phases and superconductivity in van der Waals materials.

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