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  • Letter

CuAg(SO4)2: A doubly strongly correlated altermagnetic three-dimensional analog of the parent compounds of high-Tc cuprates

Harald O. Jeschke1, Makoto Shimizu2, and Igor I. Mazin3

  • 1Research Institute for Interdisciplinary Science, Okayama University, Okayama 700-8530, Japan
  • 2Department of Physics, Graduate School of Science, Kyoto University, Kyoto 606-8502, Japan
  • 3Department of Physics and Astronomy, and Quantum Science and Engineering Center, George Mason University, Fairfax, Virginia 22030, USA

Phys. Rev. B 109, L220412 – Published 27 June, 2024

DOI: https://doi.org/10.1103/PhysRevB.109.L220412

Abstract

The discovery of high-temperature superconductivity (HTSC) in strongly correlated cuprates opened a new chapter in condensed matter physics, breaking existing stereotypes of what is a material base for a good superconductor (“Matthias rules”), at the same time emphasizing the richness and challenge of strongly correlated physics, personified by the most strongly correlated 3d ion, Cu2+. A recently reported new compound, CuAg(SO4)2, combines in a fascinating way the same ion with the most strongly correlated 4d one, Ag2+. In this Letter, we present a detailed analysis of electronic and magnetic properties of this material, and show that it is very different from the HTSC cuprates in several different ways, and opens a door into further research of superconductivity and magnetism, in particular altermagnetism, in strongly correlated materials.

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