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  • Letter

Prediction of stable nanoscale skyrmions in monolayer Fe5GeTe2

Dongzhe Li1,*, Soumyajyoti Haldar2, Leo Kollwitz2, Hendrik Schrautzer2,3, Moritz A. Goerzen2, and Stefan Heinze2,4

  • 1CEMES, Université de Toulouse, CNRS, 29 rue Jeanne Marvig, F-31055 Toulouse, France
  • 2Institute of Theoretical Physics and Astrophysics, University of Kiel, Leibnizstrasse 15, 24098 Kiel, Germany
  • 3Science Institute and Faculty of Physical Sciences, University of Iceland, VR-III, 107 Reykjavík, Iceland
  • 4Kiel Nano, Surface, and Interface Science (KiNSIS), University of Kiel, 24118 Kiel, Germany

  • *Corresponding author: dongzhe.li@cemes.fr

Phys. Rev. B 109, L220404 – Published 10 June, 2024

DOI: https://doi.org/10.1103/PhysRevB.109.L220404

Abstract

Using first-principles calculations and atomistic spin simulations, we predict stable isolated skyrmions with a diameter below 10 nm in a monolayer of the two-dimensional van der Waals ferromagnet Fe5GeTe2, a material of significant experimental interest. A very large Dzyaloshinskii-Moriya interaction (DMI) is observed due to the intrinsic broken inversion symmetry and strong spin-orbit coupling for monolayer Fe5GeTe2. We show that the nearest-neighbor approximation, often used in the literature, fails to describe the DMI. The strong DMI together with moderate in-plane magnetocrystalline anisotropy energy allows to stabilize nanoscale skyrmions in out-of-plane magnetic fields above ≈2 T. The energy barriers of skyrmions in monolayer Fe5GeTe2 are comparable to those of state-of-the-art transition-metal ultrathin films. We further predict that these nanoscale skyrmions can be stable for hours at temperatures up to 20 K.

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