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Magnetic structure of Ce3TiBi5 and its relation to current-induced magnetization

Nicolas Gauthier1,*, Romain Sibille2, Vladimir Pomjakushin2, Øystein S. Fjellvåg2,3, James Fraser4, Mathieu Desmarais4, Andrea D. Bianchi4,5, and Jeffrey A. Quilliam1

  • 1Institut Quantique, Département de physique & Regroupement Québécois sur les Matériaux de Pointe (RQMP), Université de Sherbrooke, Sherbrooke, Québec J1K 2R1, Canada
  • 2Laboratory for Neutron Scattering and Imaging, Paul Scherrer Institute, CH-5232 Villigen, Switzerland
  • 3Department for Hydrogen Technology, Institute for Energy Technology, PO Box 40, NO-2027 Kjeller, Norway
  • 4Département de Physique & Regroupement Québécois sur les Matériaux de Pointe (RQMP), Université de Montréal, Montréal, Québec H2V 0B3, Canada
  • 5Institut Courtois, Université de Montréal, Montréal, Québec H2V 0B3, Canada

  • *Corresponding author: nicolas.gauthier@inrs.ca

Phys. Rev. B 109, L140405 – Published 11 April, 2024

DOI: https://doi.org/10.1103/PhysRevB.109.L140405

Abstract

The control of magnetization using electric fields has been extensively studied in magnetoelectric multiferroic insulating materials while changes in magnetization in bulk metals caused by electric currents have attracted less attention. The recently discovered metallic magnet Ce3TiBi5 has been reported to exhibit current-induced magnetization. Here we determined the magnetic structure of Ce3TiBi5 using neutron diffraction, aiming to understand the microscopic origin of this magnetoelectric phenomenon in a metal. We established that the antiferromagnetic order emerging below TN=5K is a cycloid order described by P63/mcm.1′(0,0,g)00sss with small moment sizes of 0.50(2)μB and propagation vector k=(0,0,0.386). Surprisingly, the symmetry of this magnetic structure is inconsistent with the presence of current-induced magnetization and potential origins of this inconsistency with previous results are discussed. Additionally, our results suggest that moments order along their hard magnetic direction in Ce3TiBi5, a phenomenon which has been observed in other Kondo systems.

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