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Exciton localization on a magnetic domain wall in MoSe2−CrI3 heterostructures

S. Mikkola1, I. Chestnov1,*, I. Iorsh1,2, and V. Shahnazaryan1,2,†

  • 1Department of Physics, ITMO University, Saint Petersburg 197101, Russia
  • 2Abrikosov Center for Theoretical Physics, MIPT, Dolgoprudnyi, Moscow Region 141701, Russia

  • *igor_chestnov@mail.ru
  • †vanikshahnazaryan@gmail.com

Phys. Rev. B 108, L201403 – Published 20 November, 2023

DOI: https://doi.org/10.1103/PhysRevB.108.L201403

Abstract

The existence of spontaneous magnetization that fingerprints a ground-state ferromagnetic order was recently observed in two-dimensional (2D) van der Waals materials. Despite progress in the fabrication and manipulation of the atom-thick magnets, investigation of nanoscale magnetization properties is still challenging due to the concomitant technical issues. We propose a promising approach for a direct visualization of the domain walls formed in 2D magnetic materials. By interfacing a 2D magnet with a transition metal dichalcogenide (TMD) monolayer, the strong proximity effects enable pinning the TMD excitons on the domain wall. The emergent localization stems from the proximity-induced exchange mixing between spin-dark and spin-bright TMD excitons due to the local in-plane magnetization characteristic of the domain wall in the magnetic monolayer.

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