- Letter
Interlayer valence bonds and two-component theory for high- superconductivity of under pressure
Phys. Rev. B 108, L201108 – Published 9 November, 2023
DOI: https://doi.org/10.1103/PhysRevB.108.L201108
Abstract
The recent discovery of high- superconductivity in bilayer nickelate under high pressure has stimulated great interest concerning its pairing mechanism. We argue that the weak coupling model from the almost fully filled bonding band cannot give rise to its high , and thus propose a strong coupling model based on local interlayer spin singlets of Ni- electrons due to their strong on-site Coulomb repulsion. This leads to a minimal effective model that contains local pairing of electrons and a considerable hybridization with near quarter-filled itinerant electrons on nearest-neighbor sites. Their strong coupling provides a unique two-component scenario to achieve high- superconductivity. Our theory highlights the importance of the bilayer structure of superconducting and points out a potential route for the exploration of more high- superconductors.