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Coupling of the triple-q state to the atomic lattice by anisotropic symmetric exchange

Felix Nickel1,*, André Kubetzka2, Soumyajyoti Haldar1, Roland Wiesendanger2, Stefan Heinze1,3, and Kirsten von Bergmann2,†

  • 1Institut für Theoretische Physik und Astrophysik, Christian-Albrechts-Universität zu Kiel, D-24098 Kiel, Germany
  • 2Department of Physics, University of Hamburg, Jungiusstraße 11, 20355 Hamburg, Germany
  • 3Kiel Nano, Surface, and Interface Science (KiNSIS), University of Kiel, 24118 Kiel, Germany

  • *nickel@physik.uni-kiel.de
  • †kirsten.von.bergmann@physik.uni-hamburg.de

Phys. Rev. B 108, L180411 – Published 30 November, 2023

DOI: https://doi.org/10.1103/PhysRevB.108.L180411

Abstract

We identify the triple-q (3Q) state as magnetic ground state in Pd/Mn and Rh/Mn bilayers on Re(0001) using spin-polarized scanning tunneling microscopy and density-functional theory. An atomistic model reveals that in general the 3Q state with tetrahedral magnetic order and zero net spin moment is coupled to a hexagonal atomic lattice in a highly symmetric orientation via the anisotropic symmetric exchange interaction, whereas other spin-orbit coupling terms cancel due to symmetry. Our experiments are in agreement with the predicted orientation of the 3Q state. A distortion from the ideal tetrahedral angles would lead to other orientations of the 3Q state with a reduced topological orbital magnetization compared to the ideal 3Q state.

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