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  • Letter

Robust polaritons in magnetic monolayers of CrI3

Yaroslav Zhumagulov1,*, Salvatore Chiavazzo2, Ivan A. Shelykh3,4, and Oleksandr Kyriienko2

  • 1HSE University, Moscow 101000, Russia
  • 2Department of Physics and Astronomy, University of Exeter, Stocker Road, Exeter EX4 4QL, United Kingdom
  • 3Science Institute, University of Iceland, Dunhagi-3, IS-107 Reykjavik, Iceland
  • 4Department of Physics and Engineering, ITMO University, St. Petersburg 197101, Russia

  • *iaroslav.zhumagulov@ur.de

Phys. Rev. B 108, L161402 – Published 5 October, 2023

DOI: https://doi.org/10.1103/PhysRevB.108.L161402

Abstract

We show that the regime of strong light-matter coupling with remarkable magnetic properties can be implemented in systems based on monolayers of chromium triiodide (CrI3). This two-dimensional material combines the presence of strongly bound excitonic complexes with ferromagnetic ordering below the Curie temperature. Using microscopic first-principles calculations, we reveal a rich spectrum of optical transitions corresponding to both Wannier- and Frenkel-type excitons, including those containing electrons with an effective negative mass. We show that excitons of different polarizations efficiently hybridize with a photonic mode of a planar microcavity. Due to the peculiar selection rules, polariton modes become well resolved in circular polarizations. The strong optical oscillator strength of excitons and cavity confinement leads to large values of the Rabi splitting, reaching 35 meV for a single monolayer and giant Zeeman splitting between polariton modes of up to 20 meV. This makes CrI3 an excellent platform for magnetopolaritonic applications.

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