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Chirality-inverted Dzyaloshinskii-Moriya interaction

Khalil Zakeri1,*, Alberto Marmodoro2,3, Albrecht von Faber1, Sergiy Mankovsky4, and Hubert Ebert4

  • 1Heisenberg Spin-dynamics Group, Physikalisches Institut, Karlsruhe Institute of Technology, Wolfgang-Gaede-Strasse 1, D-76131 Karlsruhe, Germany
  • 2Institute of Physics, Academy of Science of the Czech Republic, Cukrovarnická 10, CZ-16253 Praha 6, Czech Republic
  • 3New Technologies Research Centre, University of West Bohemia, CZ-30100 Pilsen, Czech Republic
  • 4Department of Chemistry and Physical Chemistry, LMU Munich, Butenandtstrasse 11, D-81377 Munich, Germany

  • *khalil.zakeri@partner.kit.edu

Phys. Rev. B 108, L100403 – Published 19 September, 2023

DOI: https://doi.org/10.1103/PhysRevB.108.L100403

Abstract

The Dzyaloshinskii-Moriya interaction (DMI) is an antisymmetric exchange interaction, which is responsible for the formation of topologically protected spin textures in chiral magnets. Here, by measuring the dispersion relation of the DM energy, we quantify the atomistic DMI in a model system, i.e., a Co double layer on Ir(001). We unambiguously demonstrate the presence of a chirality-inverted DMI, i.e., a sign change in the chirality index of DMI from negative to positive, when comparing the interaction between nearest neighbors to that between neighbors located at longer distances. The effect is in analogy to the change in the character of the Heisenberg exchange interaction from, e.g., ferromagnetic to antiferromagnetic. We show that the pattern of the atomistic DMI in epitaxial magnetic structures can be very complex and provide critical insights into the nature of DMI. We anticipate that the observed effect is general and occurs in many magnetic nanostructures grown on heavy-element metallic substrates.

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