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Tuning heat transport in graphene by tension

H. Liu1,*, M. Lee2, M. Šiškins1,2, H. S. J. van der Zant2, P. G. Steeneken1,2, and G. J. Verbiest1,†

  • 1Department of Precision and Microsystems Engineering, Delft University of Technology, Mekelweg 2, 2628 CD Delft, The Netherlands
  • 2Kavli Institute of Nanoscience, Delft University of Technology, Lorentzweg 1, 2628 CJ Delft, The Netherlands

  • *H.Liu-7@tudelft.nl
  • †G.J.Verbiest@tudelft.nl

Phys. Rev. B 108, L081401 – Published 2 August, 2023

DOI: https://doi.org/10.1103/PhysRevB.108.L081401

Abstract

Heat transport by acoustic phonons in two-dimensional (2D) materials is fundamentally different from that in 3D crystals because the out-of-plane phonons propagate in a unique way that strongly depends on tension and bending rigidity. Here, using optomechanical techniques, we experimentally demonstrate that the heat transport time in freestanding graphene membranes is significantly higher than the theoretical prediction, and decreases by as much as 33% due to an electrostatically induced tension of 0.07 N/m. Using phonon scattering and Debye models, we explain these observations by the tension-enhanced acoustic impedance match of flexural phonons at the boundary of the graphene membrane. Thus, we experimentally elucidate the tunability of phononic heat transport in 2D materials by tension, and open a route towards electronic devices and circuits for high-speed control of temperature at the nanoscale.

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