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  • Letter

μ+ Knight shift in UTe2: Evidence for relocalization in a Kondo lattice

N. Azari1, M. R. Goeks1, M. Yakovlev1, M. Abedi1, S. R. Dunsiger1,2, S. M. Thomas3, J. D. Thompson3, P. F. S. Rosa3, and J. E. Sonier1

  • 1Department of Physics, Simon Fraser University, Burnaby, British Columbia, Canada V5A 1S6
  • 2Centre for Molecular and Materials Science, TRIUMF, Vancouver, British Columbia, Canada V6T 2A3
  • 3Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA

Phys. Rev. B 108, L081103 – Published 4 August, 2023

DOI: https://doi.org/10.1103/PhysRevB.108.L081103

Abstract

The local magnetic susceptibility of the spin-triplet superconductor UTe2 has been investigated by positive muon (μ+) Knight shift measurements in the normal state. Three distinct μ+ Knight shift components are observed for a magnetic field applied parallel to the c axis. Two of these exhibit a breakdown in the linear relationship with the bulk magnetic susceptibility (χ) below a temperature T*∼30K, which points to a gradual emergence of a correlated Kondo liquid. Below Tr∼12K linearity is gradually restored, indicating relocalization of the Kondo liquid quasiparticles. The third Knight shift component is two orders of magnitude larger, and despite the c-axis alignment of the external field, scales with the a axis χ above Tr∼12K. We conjecture that this component is associated with magnetic clusters and the change in the temperature dependence of all three Knight shift components below Tr is associated with a change in magnetic correlations. Our findings indicate that prior to the onset of superconductivity the development of the itinerant heavy-electron fluid is halted by a gradual development of local U 5f-moment fluctuations.

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