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Large upper critical fields and dimensionality crossover of superconductivity in the infinite-layer nickelate La0.8Sr0.2NiO2

Wei Wei1, Wenjie Sun2,3, Yue Sun1,*, Yongqiang Pan4, Gangjian Jin5, Feng Yang6, Yueying Li2,3, Zengwei Zhu7, Yuefeng Nie2,3,† et al.

Zhixiang Shi1,‡

  • 1Department of Physics, Southeast University, Nanjing 211189, China
  • 2National Laboratory of Solid State Microstructures, Jiangsu Key Laboratory of Artificial Functional Materials, College of Engineering and Applied Sciences, Nanjing University, Nanjing 210093, People's Republic of China
  • 3Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing 210093, People's Republic of China
  • 4Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei 230031, China
  • 5School of Electrical and Electronic Engineering, Huazhong University of Science and Technology, Wuhan 430074, China
  • 6School of Physics, Huazhong University of Science and Technology, Wuhan 430074, China
  • 7Wuhan National High Magnetic Field Center and School of Physics, Huazhong University of Science and Technology, Wuhan 430074, China

  • *Corresponding author: sunyue@seu.edu.cn
  • †Corresponding author: ynie@nju.edu.cn
  • ‡Corresponding author: zxshi@seu.edu.cn

Phys. Rev. B 107, L220503 – Published 12 June, 2023

DOI: https://doi.org/10.1103/PhysRevB.107.L220503

Abstract

The recently emerging superconductivity in infinite-layer nickelates with the isostructural and isoelectronic characteristics of cuprates provides a new platform to explore the pairing mechanism of high-temperature superconductors. In this work, we studied the upper critical field (Hc2) of a high-quality La0.8Sr0.2NiO2 thin film with superconducting transition temperature, Tconset=18.8 K, using high magnetic field up to 56 T. A very large Hc2, ∼40 T for H∥c and ∼52 T for H⊥c, was confirmed, which suggests that infinite-layer nickelates also have great application potential. The anisotropy of Hc2 monotonically decreases from ∼10(γ=Hc2ab/Hc2c) near Tc to ∼1.5 at 2 K. Angle dependence of Hc2 confirms the crossover of superconductivity from two-dimensional to three-dimensional as the temperature decreases. We discussed that the interstitial orbital effect causes the weakening of anisotropy. The observed abnormal upturning of Hc2 at low temperatures is found to be a universal behavior independent of film quality and rare-earth elements. Therefore, it should not be the Fulde-Ferrell-Larkin-Ovchinnikov state due to the fact that it is in the dirty limit and insensitive to disorder.

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