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Enhanced spin Seebeck effect in the paramagnetic phase of the three-dimensional Heisenberg antiferromagnet RbMnF3

J. D. M. de Lima, P. R. T. Ribeiro, F. L. A. Machado, and S. M. Rezende*

  • Departamento de Física, Universidade Federal de Pernambuco, 50670–901, Recife, Pernambuco, Brazil

  • *Corresponding author: sergio.rezende@ufpe.br

Phys. Rev. B 107, L140406 – Published 11 April, 2023

DOI: https://doi.org/10.1103/PhysRevB.107.L140406

Abstract

RbMnF3 is an insulating antiferromagnet with a perovskite crystal structure and Néel temperature TN=83K. Having magnetic ions with a S electronic ground state in a cubic arrangement, its magnetic anisotropy vanishes so that it is a nearly perfect three-dimensional Heisenberg antiferromagnet. Here, we report measurements of the spin Seebeck effect (SSE) in bulk samples of RbMnF3 with the shape of a slab onto which a thin Pt film strip is deposited. By applying a thermal gradient perpendicular to the slab plane, we detect an electric voltage along the Pt strip due to the charge current resulting from the conversion of the thermally generated spin current by means of the inverse spin Hall effect. By varying the magnetic field applied on the plane of the slab, we observe the antisymmetric step variation typical of the SSE both in the spin-flop and paramagnetic phases. Surprisingly the SSE increases with temperature in the paramagnetic phase and becomes comparable to the one in the ordered phase. This enhancement is attributed to a combination of the free spin fluctuations of paramagnetic insulators with the thermal conduction of long-lived paramagnons made possible by the short-range order that persists above TN.

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