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  • Letter

Field-tunable Weyl points and large anomalous Hall effect in the degenerate magnetic semiconductor EuMg2Bi2

M. Kondo1,*, M. Ochi1,2, R. Kurihara3,4, A. Miyake3, Y. Yamasaki5,6, M. Tokunaga3, H. Nakao7, K. Kuroki1, T. Kida8 et al.

M. Hagiwara8, H. Murakawa1, N. Hanasaki1,9, and H. Sakai1,†

  • 1Department of Physics, Osaka University, Toyonaka, Osaka 560-0043, Japan
  • 2Forefront Research Center, Osaka University, Toyonaka, Osaka 560-0043, Japan
  • 3The Institute for Solid State Physics, The University of Tokyo, Kashiwa, Chiba 277-8581, Japan
  • 4Department of Physics, Faculty of Science and Technology, Tokyo University of Science, Noda, Chiba 278-8510, Japan
  • 5Research and Services Division of Materials Data and Integrated System (MaDIS), National Institute for Materials Science(NIMS), Tsukuba, Ibaraki 305-0047, Japan
  • 6Center for Emergent Matter Science (CEMS), RIKEN, Wako, Saitama 351-0198, Japan
  • 7Photon Factory, Institute of Materials Structure Science, KEK, Tsukuba, Ibaraki 305-0801, Japan
  • 8Center for Advanced High Magnetic Field Science (AHMF), Graduate School of Science, Osaka University, Toyonaka, Osaka 560-0043, Japan
  • 9Spintronics Research Network Division, Institute for Open and Transdisciplinary Reserch Initiatives, Osaka University, Suita, Osaka 565-0871, Japan

  • *Corresponding author: kondo@gmr.phys.sci.osaka-u.ac.jp
  • †Corresponding author: sakai@phys.sci.osaka-u.ac.jp

Phys. Rev. B 107, L121112 – Published 28 March, 2023

DOI: https://doi.org/10.1103/PhysRevB.107.L121112

Abstract

Magnets, with topologically nontrivial Dirac/Weyl points, have recently attracted significant attention owing to their unconventional physical properties, such as a large anomalous Hall effect. However, they typically have a high carrier density and a complicated band structure near the Fermi energy. In this Letter, we report a degenerate magnetic semiconductor EuMg2Bi2, which exhibits a single valley at the Γ point, where field-tunable Weyl points form via a magnetic exchange interaction with the local Eu spins. By the high-field measurements on high-quality single crystals, we observed quantum oscillations in the resistivity, elastic constant, and surface impedance, which enabled us to determine the position of the Fermi energy EF. In combination with a first-principles calculation, we revealed that the Weyl points are located in the vicinity of EF when the Eu spins are fully polarized, leading to a peak of energy-dependent anomalous Hall conductivity due to the Berry curvature. Accordingly, in the forced ferromagnetic phase, we observed a large anomalous Hall effect (Hall angle ΘAH∼0.07) qualitatively consistent with the calculation, which demonstrates a marked impact of the Weyl points in the simple band structure.

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