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Polaron with quadratic electron-phonon interaction

Stefano Ragni1, Thomas Hahn1, Zhongjin Zhang2, Nikolay Prokof'ev2, Anatoly Kuklov3, Serghei Klimin4, Matthew Houtput4, Boris Svistunov2,5, Jacques Tempere4 et al.

Naoto Nagaosa6,7, Cesare Franchini1,8, and Andrey S. Mishchenko6

  • 1Faculty of Physics, Center for Computational Materials Science, University of Vienna, A-1090 Vienna, Austria
  • 2Department of Physics, University of Massachusetts, Amherst, Massachusetts 01003, USA
  • 3Department of Physics & Astronomy, CSI, and the Graduate Center of CUNY, New York 10314, USA
  • 4TQC, Departement Fysica, Universiteit Antwerpen, Universiteitsplein 1, B-2610 Antwerpen, Belgium
  • 5Wilczek Quantum Center, School of Physics and Astronomy and T. D. Lee Institute, Shanghai Jiao Tong University, Shanghai 200240, China
  • 6RIKEN Center for Emergent Matter Science (CEMS), 2-1 Hirosawa, Wako, Saitama 351-0198, Japan
  • 7Department of Applied Physics, The University of Tokyo 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, Japan
  • 8Dipartimento di Fisica e Astronomia, Università di Bologna, I-40127 Bologna, Italy

Phys. Rev. B 107, L121109 – Published 22 March, 2023

DOI: https://doi.org/10.1103/PhysRevB.107.L121109

Abstract

We present a numerically exact study of a polaron with quadratic coupling to the oscillator displacement, or X2 polaron, using two alternative methodological developments. Our results cover both antiadiabatic and adiabatic regimes and the entire range of electron-phonon coupling g2, from the system's stability threshold at attractive g2=−1 to arbitrary strong repulsion at g2≫1. The key properties of X2 polarons prove dramatically different from their linear counterparts. They (i) are insensitive even to large quadratic coupling except in the antiadiabatic limit near the threshold of instability at attraction, (ii) depend only on the adiabatic ratio but are insensitive to the electron dispersion and dimension of space, and (iii) feature weak lattice deformations even at the instability point. Our results are of direct relevance to the properties of electrons at low densities in polar materials, including recent proposals for their superconducting states.

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