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  • Letter

Phonon softening and slowing-down of charge density wave fluctuations in BaNi2As2

Yu Song1,2,*, Shan Wu3,4, Xiang Chen3,4, Yu He5,3,4, Hiroshi Uchiyama6, Baizhuo Li2, Saizheng Cao1, Jiayu Guo1, Guanghan Cao2 et al.

Robert Birgeneau3,4

  • 1Center for Correlated Matter and School of Physics, Zhejiang University, Hangzhou 310058, China
  • 2Zhejiang Province Key Laboratory of Quantum Technology and Device, School of Physics, Zhejiang University, Hangzhou 310058, China
  • 3Physics Department, University of California, Berkeley, California 94720, USA
  • 4Materials Science Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA
  • 5Department of Applied Physics, Yale University, New Haven, Connecticut 06511, USA
  • 6Japan Synchrotron Radiation Research Institute, SPring-8, 1-1-1 Kouto, Sayo, Hyogo 679-5198, Japan

  • *yusong_phys@zju.edu.cn

Phys. Rev. B 107, L041113 – Published 30 January, 2023

DOI: https://doi.org/10.1103/PhysRevB.107.L041113

Abstract

BaNi2As2 is a nonmagnetic analog of the iron pnictide superconductors, and exhibits an incommensurate charge density wave (IC-CDW) and a sizable elastoresistance. In this Letter, phonons in BaNi2As2 associated with the IC-CDW and uniform in-plane lattice distortions are investigated using high-resolution inelastic x-ray scattering. The in-plane transverse acoustic phonons reveal no softening at temperatures where the elastoresistance increases strongly, indicating the latter to be electronically driven. Systematic phonon measurements suggest the IC-CDW occurs in two stages upon cooling: Underdamped phonons first soften to zero energy well above the IC-CDW ordering temperature, then the resulting quasielastic IC-CDW fluctuations gradually slow down and coalesce into the static IC-CDW order. A possible origin for our observations is the IC-CDW in BaNi2As2 being uniaxial, which provides an additional Ising degree of freedom favorable for disordered IC-CDW modulations, and accounts for the elastoresistance through a weak coupling to the lattice.

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