- Editors' Suggestion
- Letter
Charge order with unusual star-of-David lattice in monolayer
Phys. Rev. B 107, L041105 – Published 17 January, 2023
DOI: https://doi.org/10.1103/PhysRevB.107.L041105
Abstract
Interplay between fermiology and electron correlation is crucial for realizing exotic quantum phases. Transition-metal dichalcogenide (TMD) has sparked tremendous attention owing to its unique Mott-insulating phase coexisting with the charge-density wave (CDW). However, how the fermiology and electron correlation are associated with such properties has yet to be clarified. Here we demonstrate that monolayer is a new class of two-dimensional TMD which has the star-of-David lattice similarly to bulk and isostructural monolayer , but exhibits a metallic ground state with an unusual lattice periodicity () characterized by the sparsely occupied star-of-David lattice. By using angle-resolved photoemission and scanning-tunneling spectroscopies in combination with first-principles band-structure calculations, we found that the hidden Fermi-surface nesting and associated CDW formation are a primary cause to realize this unique correlated metallic state with no signature of Mott gap. The present result points to a vital role of underlying fermiology to characterize the Mott phase of TMDs.