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Universality of charge doping driven metal-insulator transition in Sr2RhO4 and role of spin-orbit coupling

Junyoung Kwon1,2,*, Shoresh Soltani3,4, Craig Polley3, Jongkeun Jung1,2, Minsoo Kim1,2, Donghan Kim1,2, Jonathan Denlinger5, Dongjoon Song1,†, Yoshiyuki Yoshida6 et al.

Wonshik Kyung1,‡ and Changyoung Kim1,2,§

  • 1Center for Correlated Electron Systems, Institute for Basic Science, Seoul 08826, Korea
  • 2Department of Physics and Astronomy, Seoul National University, Seoul 08826, Korea
  • 3MAX IV Laboratory, Lund University, SE-22100 Lund, Sweden
  • 4Department of Microtechnology and Nanoscience, Chalmers University of Technology, SE-41296 Göteborg, Sweden
  • 5Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA
  • 6National Institute of Advanced Industrial Science and Technology, Tsukuba 305-8568, Japan

  • *Present address: Department of Physics, Pohang University of Science and Technology, Pohang, Gyeongbuk 37673, Korea.
  • †Present address: Stewart Blusson Quantum Matter Institute, University of British Columbia, Vancouver, British Columbia V6T 1Z1, Canada.
  • ‡specialtoss@gmail.com
  • §changyoung@snu.ac.kr

Phys. Rev. B 106, L241114 – Published 30 December, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L241114

Abstract

We performed angle-resolved photoemission spectroscopy (ARPES) experiments on an electron-doped Sr2RhO4 system Sr2−xCexRhO4 in order to investigate the electron doping-induced metal-insulator transition (MIT). We establish the universality of MIT in electron-doped Sr2RhO4 by comparing results from Sr2−xLaxRhO4 and Sr2−xCexRhO4. Via a systematic analysis of doping-dependent transport and ARPES data, we show that the correlation driven MIT with a noninteger electron number in electron-doped Sr2RhO4 is universal and thus independent of the dopant. Within the universality, the ARPES analysis shows that the band topology determined by the spin-orbit coupling (SOC) is likely a control parameter of the insulating gap size and critical electron number of the MIT. We present a phase diagram of the insulating phase as a function of the effective SOC and electron number.

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