- Letter
Effect of magnetism and phonons on localized carriers in the ferrimagnetic kagome metals and
Phys. Rev. B 106, L241108 – Published 19 December, 2022
DOI: https://doi.org/10.1103/PhysRevB.106.L241108
Abstract
Kagome metals possess peculiar optical spectra consisting of contributions from free charge carriers in a Drude-type response, localized carriers seen as a strongly temperature-dependent localization peak, and, in some cases, phonons displaying strong anomalies. The rare-earth kagome metal series, , provides a marvelous playground to study the electronic properties of kagome metals in the presence of variable magnetic order. Here, we report temperature-dependent reflectivity studies on two members of the family, (in-plane ferrimagnet) and (out-of-plane ferrimagnet), in a broad energy range (50–18 000 , equivalent to 6.2 meV–2.23 eV) down to 10 K. At high temperatures, a phonon mode at approximately 160 is observed, which becomes screened out in below 150 K as the localization peak linearly passes through the mode. In , the disappearance of the phonon is accompanied by the onset of saturation of the peak position, suggesting an unusual interplay between the two features.