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Effect of magnetism and phonons on localized carriers in the ferrimagnetic kagome metals GdMn6Sn6 and TbMn6Sn6

M. Wenzel1,*, A. A. Tsirlin2,3, O. Iakutkina1, Q. Yin4, H. C. Lei4, M. Dressel1, and E. Uykur1,5

  • 11. Physikalisches Institut, Universität Stuttgart, 70569 Stuttgart, Germany
  • 2Felix Bloch Institute for Solid-State Physics, Leipzig University, 04103 Leipzig, Germany
  • 3Experimental Physics VI, Center for Electronic Correlations and Magnetism, Institute of Physics, University of Augsburg, 86135 Augsburg, Germany
  • 4Laboratory for Neutron Scattering, and Beijing Key Laboratory of Optoelectronic Functional Materials MicroNano Devices, Department of Physics, Renmin University of China, Beijing 100872, China
  • 5Helmholtz-Zentrum Dresden-Rossendorf, Institute of Ion Beam Physics and Materials Research, 01328 Dresden, Germany

  • *maxim.wenzel@pi1.physik.uni-stuttgart.de

Phys. Rev. B 106, L241108 – Published 19 December, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L241108

Abstract

Kagome metals possess peculiar optical spectra consisting of contributions from free charge carriers in a Drude-type response, localized carriers seen as a strongly temperature-dependent localization peak, and, in some cases, phonons displaying strong anomalies. The rare-earth kagome metal series, RMn6Sn6, provides a marvelous playground to study the electronic properties of kagome metals in the presence of variable magnetic order. Here, we report temperature-dependent reflectivity studies on two members of the RMn6Sn6 family, GdMn6Sn6 (in-plane ferrimagnet) and TbMn6Sn6 (out-of-plane ferrimagnet), in a broad energy range (50–18 000 cm−1, equivalent to 6.2 meV–2.23 eV) down to 10 K. At high temperatures, a phonon mode at approximately 160 cm−1 is observed, which becomes screened out in TbMn6Sn6 below ∼150 K as the localization peak linearly passes through the mode. In GdMn6Sn6, the disappearance of the phonon is accompanied by the onset of saturation of the peak position, suggesting an unusual interplay between the two features.

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