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  • Letter

Stacking-induced magnetic frustration and spiral spin liquid

Jianqiao Liu1,*, Xu-Ping Yao2,*, and Gang Chen2,3,†

  • 1State Key Laboratory of Surface Physics and Department of Physics, Fudan University, Shanghai 200433, China
  • 2Department of Physics and HKU-UCAS Joint Institute for Theoretical and Computational Physics at Hong Kong, The University of Hong Kong, Hong Kong, China
  • 3The University of Hong Kong Shenzhen Institute of Research and Innovation, Shenzhen 518057, China

  • *These authors contributed equally to this work.
  • †gangchen@hku.hk

Phys. Rev. B 106, L220410 – Published 29 December, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L220410

Abstract

Like the twisting control in magic-angle twisted bilayer graphene, the stacking control is another mechanical approach to manipulate the fundamental properties of solids, especially the van der Waals materials. We explore the stacking-induced magnetic frustration and the spiral spin liquid on a multilayer triangular lattice antiferromagnet where the system is built from ABC stacking with competing intralayer and interlayers couplings. By combining the nematic bond theory and the self-consistent Gaussian approximation, we establish the phase diagram for this ABC-stacked multilayer magnet. It is shown that the system supports a wide regime of spiral spin liquid with multiple degenerate spiral lines in the reciprocal space, separating the low-temperature spiral order and the high-temperature featureless paramagnet. The transition to the spiral order from the spiral spin liquid regime is first order. We further show that the spiral-spin-liquid behavior persists even with small perturbations such as further neighbor intralayer exchanges. The connection to the ABC-stacked magnets, the effects of Ising or planar spin anisotropy, and the outlook on the stacking-engineered quantum magnets are discussed.

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