- Letter
Glassy electrons at the first-order Mott metal-insulator transition
Phys. Rev. B 106, L201112 – Published 23 November, 2022
DOI: https://doi.org/10.1103/PhysRevB.106.L201112
Abstract
The Mott metal-insulator transition remains one of the most scrutinized concepts in condensed matter physics. However, the kinetics of the charge carriers at the transition, involving both orbital and spin degrees of freedom, still remains poorly understood. A perfect platform to distinguish between the role of such competing interactions is strongly correlated oxides offering rich phase diagrams, which we use here to address the electron kinetics at the transition. We show a critical slowing down of the electron kinetics at the first-order Mott metal-insulator transition in the Ruddlesden-Popper oxide using low-frequency noise in resistance fluctuations. A critical slowing down of the electron kinetics is manifested as an enhancement of noise by an order of magnitude at the transition with a large shift of the spectral weight to lower frequencies. The second spectrum of noise is frequency dependent, indicating the presence of correlated fluctuations which get suppressed under the application of a magnetic field. Our experiments provide compelling evidence of the formation of a spin-glass phase at the transition in these systems.
Physics Subject Headings (PhySH)
Corrections
2 December, 2022
Correction: The “Corresponding author” identifier was removed from the byline footnote for the second author during the proof production process and has been restored.