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  • Letter

Tunable electronic and magnetic phases in layered ruthenates: Strained SrRuO3−SrTiO3 heterostructures

Minjae Kim1,*, Chang-Jong Kang2,†, Jae-Ho Han3, Kyoo Kim4, and Bongjae Kim5,‡

  • 1Korea Institute for Advanced Study, Seoul 02455, South Korea
  • 2Department of Physics, Chungnam National University, Daejeon 34134, South Korea
  • 3Center for Theoretical Physics of Complex Systems, Institute for Basic Science (IBS), Daejeon 34126, South Korea
  • 4Korea Atomic Energy Research Institute (KAERI), Daejeon 34057, South Korea
  • 5Department of Physics, Kunsan National University, Gunsan 54150, South Korea

  • *garix.minjae.kim@gmail.com
  • †cjkang87@cnu.ac.kr
  • ‡bongjae.kim@kunsan.ac.kr

Phys. Rev. B 106, L201103 – Published 3 November, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L201103

Abstract

Layered ruthenates are a unique class of systems which manifest a variety of electronic and magnetic features from competing energy scales. At the heart of such features lies multi-orbital physics, especially orbital-selective behavior. Here, we propose that the SrRuO3−SrTiO3 heterostructure is a highly tunable platform to obtain the various emergent properties. Employing the density functional theory plus dynamical mean-field theory, we thoroughly investigate the orbital-dependent physics of the system and identify the competing magnetic fluctuations. We show that the epitaxial strain drives the system towards multi-orbital or orbital selective Mott phases from the Hund metal regime. At the same time, the two different types of static magnetism, ferromagnetism and checkerboard antiferromagnetism, are stabilized from the competition with the spin-density wave instability.

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