Export citation

Export citation

Choose format for download:

Download Citation
  • Editors' Suggestion
  • Letter

Antiferromagnetic fluctuations and orbital-selective Mott transition in the van der Waals ferromagnet Fe3−xGeTe2

Xiaojian Bai1,*, Frank Lechermann2,†, Yaohua Liu1, Yongqiang Cheng1, Alexander I. Kolesnikov1, Feng Ye1, Travis J. Williams1, Songxue Chi1, Tao Hong1 et al.

Garrett E. Granroth1, Andrew F. May3, and Stuart Calder1,‡

  • 1Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA
  • 2Institut für Theoretische Physik III, Ruhr-Universität Bochum, D-44780 Bochum, Germany
  • 3Materials Science & Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, USA

  • *baix@ornl.gov
  • †frank.lechermann@ruhr-uni-bochum.de
  • ‡caldersa@ornl.gov

Phys. Rev. B 106, L180409 – Published 30 November, 2022

DOI: https://doi.org/10.1103/PhysRevB.106.L180409

Abstract

Fe3−xGeTe2 is a layered magnetic van der Waals material of interest for both fundamental and applied research. Despite the observation of intriguing physical properties, open questions exist even on the basic features related to magnetism: is it a simple ferromagnet or are there antiferromagnetic regimes, and are the moments local or itinerant. Here, we demonstrate that antiferromagnetic spin fluctuations coexist with the ferromagnetism through comprehensive elastic and inelastic neutron scattering and thermodynamic measurements. Our realistic dynamical mean-field theory calculations reveal that the competing magnetic fluctuations are driven by an orbital selective Mott transition (OSMT), where only the plane-perpendicular a1g orbital of the Fe(3d) manifold remains itinerant. Our results highlight the multi-orbital character in Fe3−xGeTe2 that supports a rare coexistence of local and itinerant physics within this material.

Physics Subject Headings (PhySH)

Authorization Required

We need you to provide your credentials before accessing this content.

Supplemental Material (Subscription Required)

References (Subscription Required)

Outline

Information

Sign In to Your Journals Account

Filter

Filter

Article Lookup

Enter a citation